Howes C, Saide PE, Coe H, Dobracki A, Freitag S, Haywood JM, Howell SG, Gupta S, Uin J, Kacarab M, et al. Biomass-burning smoke's properties and its interactions with marine stratocumulus clouds in WRF-CAM5 and southeastern Atlantic field campaigns. Atmospheric Chemistry and Physics [Internet]. 2023;23 (21) :13911–13940. Publisher's Version
Saide PE, Krishna M, Ye X, Thapa LH, Turney F, Howes C, Schmidt CC. Estimating Fire Radiative Power Using Weather Radar Products for Wildfires. Geophysical Research Letters [Internet]. 2023;50 (21) :e2023GL104824. Publisher's VersionAbstract
Abstract Satellite-based Fire radiative power (FRP) retrievals are used to track wildfire activity but are sometimes not possible or have large uncertainties. Here, we show that weather radar products including composite and base reflectivity and equivalent rainfall integrated in the vicinity of the fires show strong correlation with hourly FRP for multiple fires during 2019–2020. Correlation decreases when radar beams are blocked by topography and when there is significant ground clutter (GC) and anomalous propagation (AP). GC/AP can be effectively removed using a machine learning classifier trained with radar retrieved correlation coefficient, velocity, and spectrum width. We find a power-law best describes the relationship between radar products and FRP for multiple fires combined (0.67–0.76 R2). Radar-based FRP estimates can be used to fill gaps in satellite FRP created by cloud cover and show great potential to overcome satellite FRP biases occurring during extreme fire events.
Pagonis D, Selimovic V, Campuzano-Jost P, Guo H, Day DA, Schueneman MK, Nault BA, Coggon MM, DiGangi JP, Diskin GS, et al. Impact of Biomass Burning Organic Aerosol Volatility on Smoke Concentrations Downwind of Fires. Environmental Science & Technology. 2023.
Turney FA, Saide PE, Jimenez Munoz PA, Muñoz-Esparza D, Hyer EJ, Peterson DA, Frediani ME, Juliano TW, DeCastro AL, Kosović B, et al. Sensitivity of Burned Area and Fire Radiative Power Predictions to Containment Efforts, Fuel Density, and Fuel Moisture Using WRF-Fire. Journal of Geophysical Research: Atmospheres [Internet]. 2023;128 (18) :e2023JD038873. Publisher's VersionAbstract
Abstract Predicting the evolution of burned area, smoke emissions, and energy release from wildfires is crucial to air quality forecasting and emergency response planning yet has long posed a significant scientific challenge. Here we compare predictions of burned area and fire radiative power from the coupled weather/fire-spread model WRF-Fire (Weather and Research Forecasting Tool with fire code), against simpler methods typically used in air quality forecasts. We choose the 2019 Williams Flats Fire as our test case due to a wealth of observations and ignite the fire on different days and under different configurations. Using a novel re-gridding scheme, we compare WRF-Fire's heat output to geostationary satellite data at 1-hr temporal resolution. We also evaluate WRF-Fire's time-resolved burned area against high-resolution imaging from the National Infrared Operations aircraft data. Results indicate that for this study, accounting for containment efforts in WRF-Fire simulations makes the biggest difference in achieving accurate results for daily burned area predictions. When incorporating novel containment line inputs, fuel density increases, and fuel moisture observations into the model, the error in average daily burned area is 30% lower than persistence forecasting over a 5-day forecast. Prescribed diurnal cycles and those resolved by WRF-Fire simulations show a phase offset of at least an hour ahead of observations, likely indicating the need for dynamic fuel moisture schemes. This work shows that with proper configuration and input data, coupled weather/fire-spread modeling has the potential to improve smoke emission forecasts.
Tang B, Saide PE, Gao M, Carmichael GR, Stanier CO. WRF-Chem quantification of transport events and emissions sensitivity in Korea during KORUS-AQ. Elementa: Science of the Anthropocene [Internet]. 2023;11 (1). Publisher's VersionAbstract
To quantify the relative roles of long-range transport (LRT) versus locally emitted aerosol and ozone precursors during polluted periods in Korea, high-resolution (4 km) Weather Research and Forecasting with Chemistry model simulations were performed. The model was evaluated using surface and airborne observations collected during the KORea and United States Air Quality campaign. Ozone above 40 ppb had mean bias of −5.9 ppb. PM2.5 was biased high (8.2 µg/m3), with a relative bias of 30\% given the mean observed value of 26.8 µg/m3. The absolute amounts and shifts between phases for all PM2.5 species except nitrate reasonably match observations across all 4 phases. Notable limitations include an underestimation of nighttime planetary boundary layer height. Transport versus domestic emissions influence was studied by model runs with perturbed emissions and by comparing east-west fluxes over the Yellow Sea to Korean emissions and other normalization metrics. Domestic anthropogenic emission contributions to surface air quality were quantified by location across Korea, segregated by synoptic meteorological phase. The largest contributions from Korean emissions were found under high-pressure stagnant conditions and the smallest for conditions with strong westerly winds. For example, at Seoul, domestic contributions of PM2.5 averaged 49\% and 29\% in the aforementioned meteorological phases, respectively. Surface concentrations of NOx and toluene in Seoul were over 85\% due to domestic emissions. CO and black carbon had both local and remote contributions. Nitrate and ammonium contributions varied greatly by phases in Seoul, with 7\%–51\% nitrate and 42\%–70\% of ammonium from remote sources. Variation in direction (west-to-east vs. east-to-west) and magnitude of fluxes support the model sensitivity results. Analysis using fluxes facilitates the quantification of source contributions for secondary species and, in many cases, can be done using a single model run or reanalysis result. The analysis presented shows the importance of using models with high spatial resolution to capture pollutant transport and mixing around Korea. However, there remain uncertainties in secondary aerosol production mechanisms and indications that local production at times could be higher than those modeled in this analysis. Therefore, the results presented here should be viewed as an upper limit on the importance of LRT.
Yu J, Song CH, Lee D, Lee S, Kim HS, Han KM, Park S, Im J, Park S-Y, Jeon M, et al. Synergistic combination of information from ground observations, geostationary satellite, and air quality modeling towards improved PM2. 5 predictability. npj Climate and Atmospheric Science. 2023;6 (1) :41.
Berman M, Ye X, Thapa L, Peterson DA, Hyer E, Soja A, Gargulinski E, Csiszar I, Schmidt C, Saide P. Quantifying burned area of wildfires in the Western United States from polar-orbiting and geostationary satellite active-fire detections. International Journal of Wildland Fire [Internet]. 2023. Publisher's Version
Dobracki A, Zuidema P, Howell SG, Saide P, Freitag S, Aiken AC, Burton SP, Sedlacek III AJ, Redemann J, Wood R. An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic. Atmospheric Chemistry and Physics [Internet]. 2023;23 (8) :4775–4799. Publisher's Version
Lenhardt ED, Gao L, Redemann J, Xu F, Burton SP, Cairns B, Chang I, Ferrare RA, Hostetler CA, Saide PE, et al. Use of lidar aerosol extinction and backscatter coefficients to estimate cloud condensation nuclei (CCN) concentrations in the southeast Atlantic. Atmospheric Measurement Techniques [Internet]. 2023;16 (7) :2037–2054. Publisher's Version
Chang I, Gao L, Flynn CJ, Shinozuka Y, Doherty SJ, Diamond MS, Longo KM, Ferrada GA, Carmichael GR, Castellanos P, et al. On the differences in the vertical distribution of modeled aerosol optical depth over the southeastern Atlantic. Atmospheric Chemistry and Physics [Internet]. 2023;23 (7) :4283–4309. Publisher's Version
Warneke C, Schwarz JP, Dibb J, Kalashnikova O, Frost G, Al-Saad J, Brown SS, Brewer WA, Soja A, Seidel FC, et al. Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ). Journal of Geophysical Research: Atmospheres [Internet]. 2023;128 (2) :e2022JD037758. Publisher's VersionAbstract
Abstract The NOAA/NASA Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) experiment was a multi-agency, inter-disciplinary research effort to: (a) obtain detailed measurements of trace gas and aerosol emissions from wildfires and prescribed fires using aircraft, satellites and ground-based instruments, (b) make extensive suborbital remote sensing measurements of fire dynamics, (c) assess local, regional, and global modeling of fires, and (d) strengthen connections to observables on the ground such as fuels and fuel consumption and satellite products such as burned area and fire radiative power. From Boise, ID western wildfires were studied with the NASA DC-8 and two NOAA Twin Otter aircraft. The high-altitude NASA ER-2 was deployed from Palmdale, CA to observe some of these fires in conjunction with satellite overpasses and the other aircraft. Further research was conducted on three mobile laboratories and ground sites, and 17 different modeling forecast and analyses products for fire, fuels and air quality and climate implications. From Salina, KS the DC-8 investigated 87 smaller fires in the Southeast with remote and in-situ data collection. Sampling by all platforms was designed to measure emissions of trace gases and aerosols with multiple transects to capture the chemical transformation of these emissions and perform remote sensing observations of fire and smoke plumes under day and night conditions. The emissions were linked to fuels consumed and fire radiative power using orbital and suborbital remote sensing observations collected during overflights of the fires and smoke plumes and ground sampling of fuels.
Ye X, Deshler M, Lyapustin A, Wang Y, Kondragunta S, Saide P. Assessment of Satellite AOD during the 2020 Wildfire Season in the Western U.S. Remote Sensing [Internet]. 2022;14 (23). Publisher's VersionAbstract
Satellite remote sensing of aerosol optical depth (AOD) is essential for detection, characterization, and forecasting of wildfire smoke. In this work, we evaluate the AOD (550 nm) retrievals during the extreme wildfire events over the western U.S. in September 2020. Three products are analyzed, including the Moderate-resolution Imaging Spectroradiometers (MODIS) Multi-Angle Implementation of Atmospheric Correction (MAIAC) product collections C6.0 and C6.1, and the NOAA-20 Visible Infrared Imaging Radiometer (VIIRS) AOD from the NOAA Enterprise Processing System (EPS) algorithm. Compared with the Aerosol Robotic Network (AERONET) data, all three products show strong linear correlations with MAIAC C6.1 and VIIRS presenting overall low bias (<0.06). The accuracy of MAIAC C6.1 is found to be substantially improved with respect to MAIAC C6.0 that drastically underestimated AOD over thick smoke, which validates the effectiveness of updates made in MAIAC C6.1 in terms of an improved representation of smoke aerosol optical properties. VIIRS AOD exhibits comparable uncertainty with MAIAC C6.1 with a slight tendency of increased positive bias over the AERONET AOD range of 0.5–3.0. Averaging coincident retrievals from MAIAC C6.1 and VIIRS provides a lower root mean square error and higher correlation than for the individual products, motivating the benefit of blending these datasets. MAIAC C6.1 and VIIRS are further compared to provide insights on their retrieval strategy. When gridded at 0.1° resolution, MAIAC C6.1 and VIIRS provide similar monthly AOD distribution patterns and the latter exhibits a slightly higher domain average. On daily scale, over thick plumes near fire sources, MAIAC C6.1 reports more valid retrievals where VIIRS tends to have retrievals designated as low or medium quality, which tends to be due to internal quality checks. Over transported smoke near scattered clouds, VIIRS provides better retrieval coverage than MAIAC C6.1 owing to its higher spatial resolution, pixel-level processing, and less strict cloud masking. These results can be used as a guide for applications of satellite AOD retrievals during wildfire events and provide insights on future improvement of retrieval algorithms under heavy smoke conditions.
Thapa LH, Ye X, Hair JW, Fenn MA, Shingler T, Kondragunta S, Ichoku C, Dominguez RA, Ellison L, Soja AJ, et al. Heat flux assumptions contribute to overestimation of wildfire smoke injection into the free troposphere. Communications Earth & Environment [Internet]. 2022;3 (1) :1–11. Publisher's Version
Ye X, Saide PE, Hair J, Fenn M, Shingler T, Soja A, Gargulinski E, Wiggins E. Assessing Vertical Allocation of Wildfire Smoke Emissions Using Observational Constraints From Airborne Lidar in the Western U.S. Journal of Geophysical Research: Atmospheres [Internet]. 2022;127 (21) :e2022JD036808. Publisher's VersionAbstract
Abstract Wildfire emissions are a key contributor of carbonaceous aerosols and trace gases to the atmosphere. Induced by buoyant lifting, smoke plumes can be injected into the free troposphere and lower stratosphere, which by consequence significantly affects the magnitude and distance of their influences on air quality and radiation budget. However, the vertical allocation of emissions when smoke escapes the planetary boundary layer (PBL) and the mechanism modulating it remain unclear. We present an inverse modeling framework to estimate the wildfire emissions, with their temporal and vertical evolution being constrained by assimilating aerosol extinction profiles observed from the airborne Differential Absorption Lidar-High Spectral Resolution Lidar during the Fire Influence on Regional to Global Environments and Air Quality field campaign. Three fire events in the western U.S., which exhibit free-tropospheric injections are examined. The constrained smoke emissions indicate considerably larger fractions of smoke injected above the PBL (f>PBL, 80%–94%) versus the column total, compared to those estimated by the WRF-Chem model using the default plume rise option (12%–52%). The updated emission profiles yield improvements for the simulated vertical structures of the downwind transported smoke, but limited refinement of regional smoke aerosol optical depth distributions due to the spatiotemporal coverage of flight observations. These results highlight the significance of improving vertical allocation of fire emissions on advancing the modeling and forecasting of the environmental impacts of smoke.
Saide PE, Thapa LH, Ye X, Pagonis D, Campuzano-Jost P, Guo H, Schuneman ML, Jimenez J-L, Moore R, Wiggins E, et al. Understanding the Evolution of Smoke Mass Extinction Efficiency Using Field Campaign Measurements. Geophysical Research Letters [Internet]. 2022;49 (18) :e2022GL099175. Publisher's VersionAbstract
Abstract Aerosol mass extinction efficiency (MEE) is a key aerosol property used to connect aerosol optical properties with aerosol mass concentrations. Using measurements of smoke obtained during the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign we find that mid-visible smoke MEE can change by a factor of 2–3 between fresh smoke (<2 hr old) and one-day-old smoke. While increases in aerosol size partially explain this trend, changes in the real part of the aerosol refractive index (real(n)) are necessary to provide closure assuming Mie theory. Real(n) estimates derived from multiple days of FIREX-AQ measurements increase with age (from 1.40 – 1.45 to 1.5–1.54 from fresh to one-day-old) and are found to be positively correlated with organic aerosol oxidation state and aerosol size, and negatively correlated with smoke volatility. Future laboratory, field, and modeling studies should focus on better understanding and parameterizing these relationships to fully represent smoke aging.
Lee S, Song CH, Han KM, Henze DK, Lee K, Yu J, Woo J-H, Jung J, Choi Y, Saide PE, et al. Impacts of uncertainties in emissions on aerosol data assimilation and short-term PM2.5 predictions over Northeast Asia. Atmospheric Environment [Internet]. 2022;271 :118921. Publisher's VersionAbstract
To improve PM2.5 predictions in Northeast Asia, we estimated a new background error covariance matrix (BEC) for aerosol data assimilation using surface PM2.5 observations. In contrast to the conventional method of BEC estimation that uses perturbations in meteorological data, this method additionally considered the perturbations using two different emission inventories. By taking the emission uncertainty into account, we found that the standard deviations in the BEC were significantly increased. The standard deviations became around three times larger than those in the conventional method at the surface. The impacts of the new BEC were then tested for the prediction of surface PM2.5 over Northeast Asia using the Community Multiscale Air Quality (CMAQ) model initialized by three-dimensional variational method (3D-VAR). The surface PM2.5 data measured at 154 sites in South Korea and 1535 sites in China were assimilated every 6 h during the campaign period of the Korea-United States Air Quality Study (KORUS-AQ) (1 May–14 June 2016). The data assimilation with the new BEC showed better agreement with the surface PM2.5 observations than with the BEC from the conventional method. Our method was also more consistent with the observations in 24-h PM2.5 predictions than the conventional method (specifically, with a ∼44% reduction of negative biases). We concluded that increased standard deviations, together with updated horizontal and vertical length scales in the new BEC, improved the data assimilation and short-term predictions of the surface PM2.5. This paper also suggests several research efforts to further improve the BEC for better short-term PM2.5 predictions in Northeast Asia.
Diamond MS, Saide PE, Zuidema P, Ackerman AS, Doherty SJ, Fridlind AM, Gordon H, Howes C, Kazil J, Yamaguchi T, et al. Cloud adjustments from large-scale smoke–circulation interactions strongly modulate the southeastern Atlantic stratocumulus-to-cumulus transition. Atmospheric Chemistry and Physics [Internet]. 2022;22 (18) :12113–12151. Publisher's Version
Peterson DA, Thapa LH, Saide PE, Soja AJ, Gargulinski EM, Hyer EJ, Weinzierl B, Dollner M, Schöberl M, Papin PP, et al. Measurements from inside a Thunderstorm Driven by Wildfire: The 2019 FIREX-AQ Field Experiment. Bulletin of the American Meteorological Society [Internet]. 2022. Publisher's Version
Doherty SJ, Saide PE, Zuidema P, Shinozuka Y, Ferrada GA, Gordon H, Mallet M, Meyer K, Painemal D, Howell SG, et al. Modeled and observed properties related to the direct aerosol radiative effect of biomass burning aerosol over the southeastern Atlantic. Atmospheric Chemistry and Physics [Internet]. 2022;22 (1) :1–46. Publisher's Version
Ye X, Arab P, Ahmadov R, James E, Grell GA, Pierce B, Kumar A, Makar P, Chen J, Davignon D, et al. Evaluation and intercomparison of wildfire smoke forecasts from multiple modeling systems for the 2019 Williams Flats fire. Atmospheric Chemistry and Physics [Internet]. 2021;21 (18) :14427–14469. Publisher's Version